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Closed-Form Calculation of Coherent Anti-Stokes Raman and Stimulated Raman Scattering Spectral Profiles

Volume 35, Number 3 (June 1981) Page 276-278

Perkins, P.E.; Lewis, J.W.L.

The third-order susceptibility is expressed as a summation of interfering resonant terms, each involving the phenomenological linewidth of the transition. Correlations of the finite line-width of the laser sources with |X(3)|2 (coherent anti-Stokes Raman spectroscopy) and -X" (stimulated Raman scattering) are performed and closed-form expressions for the theoretical profiles are obtained.