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Interpretation Coherent Anti-Stokes Raman Spectroscopy (CARS) Spectral Profiles

Volume 33, Number 3 (June 1979) Page 268-273

Shaub, W.M.; Lemont, S.; Harvey, A.B.


CARS spectral profiles are functionally described by the variation of the square of the total third-order, nonlinear susceptibility with the anti-Stokes frequency shift. This inherent, squared susceptibility signal dependence, when weighted by an experiment dependent convolution, produces a CARS spectral profile which is a problem specific to the experiment design.